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Sr (
Sr) from port of Fukushima Daiichi Nuclear Power Plant; Analysis of the temporal variation from the accident to March 2022 and evaluation of its impact on Fukushima coast and offshore areasMachida, Masahiko; Iwata, Ayako; Yamada, Susumu; Otosaka, Shigeyoshi*; Kobayashi, Takuya; Funasaka, Hideyuki*; Morita, Takami*
Nihon Genshiryoku Gakkai Wabun Rombunshi (Internet), 22(4), p.119 - 139, 2023/11
We estimate monthly discharged inventory of Sr from port of Fukushima Daiichi Nuclear Power Plant (1F) from Jun. 2013 to Mar. 2022 by using the Voronoi tessellation method inside the port, following the monitoring of Sr sea water radioactivity concentration inside the port. The results suggest that the closure of sea side impermeable wall is the most effective for the reduction of discharged one. In addition, the results roughly reveal the monthly discharged inventory required to observe visible enhancement of the sea radioactivity concentration from the background level in each area. Such outcome is significant for considering environmental impacts on the planned future releasing of the treated water accumulated in 1F site.
Ono, Ayato; Takayanagi, Tomohiro; Sugita, Moe; Ueno, Tomoaki*; Horino, Koki*; Yamamoto, Kazami; Kinsho, Michikazu
JAEA-Technology 2022-036, 31 Pages, 2023/03
JAEA-Technology-2022-036.pdf:8.77MB
In the Japan Atomic Energy Agency (JAEA), many electrical facilities such as power receiving equipment and power supply units are installed in experimental facilities such as the Nuclear Science Research Institute (NSRI) and the Japan Proton Accelerator Research Complex (J-PARC). However, some facilities have been in operation for more than half a century since they were manufactured, some have already been closed or deactivated, and others are still in operation while replacing parts and taking other aging measures. In these facilities, materials that were used because of their excellent properties at the time of manufacture are now designated as hazardous substances and require special management when disposed of. One of them is polychlorinated biphenyl (PCB). PCB were used in a very wide range of fields because of their stability against heat, high electrical insulation, and chemical resistance. However, it was found that PCB have persistent properties and may cause damage to human health and the living environment, and the government has enacted the "Act on Special Measures for Promotion of Proper Treatment of PCB Wastes (PCB Special Measures Law)" to promote reliable and proper disposal. JAEA has almost completed the excavation survey of high-concentration PCB waste and is in the process of excavating low-concentration PCB waste. However, there are still new relevant items to be discovered. This report summarizes and reports the knowledge necessary for identifying PCB waste and points to be noted when handling capacitors, etc., based on examples of actual disassembly and investigation work conducted on power supply units and other electrical equipment, such as capacitors attached to power supply units, etc.
Oka, Hiroshi*; Tanno, Takashi; Yano, Yasuhide; Otsuka, Satoshi; Kaito, Takeji; Hashimoto, Naoyuki*
Journal of Nuclear Materials, 572, p.154032_1 - 154032_8, 2022/12
Times Cited Count：3 Percentile：68.71(Materials Science, Multidisciplinary)9Cr oxide dispersion strengthened steels with slightly different nitrogen concentrations (0.0034 - 0.029 wt%) were prepared and their creep property at 973 K was investigated with microstructural characterization before and after the creep test. The creep strength decreased significantly as the nitrogen concentration increased. Microstructural observation revealed that, in the higher nitrogen concentration specimen, coarse Y-rich inclusions were found along the boundary between transformed ferrite region and residual ferrite region. The solubility difference of nitrogen in 
and 
phase would induce the localized increment of nitrogen concentration in the boundary region during the austenitizing process, resulting in the thermodynamic destabilization and subsequent coarsening of the dispersed oxide particles. The rows of creep voids were found near the rupture part of the crept specimen, suggesting that the coarse inclusions were the starting point of creep void formation and the subsequent premature fracture.
Okada, Shota; Murakami, Masashi; Kochiyama, Mami; Izumo, Sari; Sakai, Akihiro
JAEA-Testing 2022-002, 66 Pages, 2022/08
JAEA-Testing-2022-002.pdf:2.46MB
Japan Atomic Energy Agency is an implementing organization of burial disposal for low-level radioactive waste generated from research, industrial and medical facilities in Japan. Radioactivity concentrations of the waste are essential information for design of the disposal facility and for licensing process. A lot of the waste subjected to the burial disposal is arising from dismantling of nuclear facilities. Radioactive Wastes Disposal enter has therefore discussed a procedure to evaluate the radioactivity concentrations by theoretical calculation for waste arising from the dismantling of the research reactors facilities and summarized the common procedure. The procedure includes evaluation of radioactive inventory by activation calculation, validation of the calculation results, and determination of the disposal classification as well as organization of the data on total radioactivity and maximum radioactivity concentration for each classification. For the evaluation of radioactive inventory, neutron flux and energy spectra are calculated at each region in the reactor facility using two- or three-dimensional neutron transport code. The activation calculation is then conducted for 140 nuclides using the results of neutron transport calculation and an activation calculation code. The recommended codes in this report for neutron transport calculation are two-dimensional discrete ordinate code DORT, three-dimensional discrete ordinate code TORT, or Monte Carlo codes MCNP and PHITS, and for activation calculation is ORIGEN-S. Other recommendation of cross-section libraries and calculation conditions are also indicated in this report. In the course of the establishment of the procedure, Radioactive Wastes Disposal Center has discussed the commonly available procedure at meetings. It has periodically held to exchange information with external operators which have research reactor facilities. The procedure will properly be reviewed and be revised by reflecting future situ
Sakuma, Kota; Abe, Daichi*; Okada, Shota; Sugaya, Toshikatsu; Nakata, Hisakazu; Sakai, Akihiro
JAEA-Technology 2022-013, 200 Pages, 2022/08
JAEA-Technology-2022-013.pdf:8.41MB
Japan Atomic Energy Agency has aims to carry out near surface disposal of low-level radioactive waste generated from research, medical, and industrial facilities. Therefore, Radioactivity Concentration Corresponding to Dose Criterion for near surface disposal for nuclides in the waste were calculated for the purpose of discussion for radioactivity limits between trench and concrete vault disposal, and key nuclides related to them. This report uses the results of sensitivity analysis and evaluation of the amount of leachate from the disposal facility for concrete vault disposal, and incorporates a new assessment pathway and exposure form that widely assume the conditions of the disposal facility. This trial calculation was carried out and compared with the trial calculation in the previous report, "Evaluation of Radioactivity Concentration Corresponding to Dose Criterion for Near Surface Disposal of Radioactive Waste Generated from Research, Medical, and Industrial Facilities, Volume 1". The results of Radioactivity Concentration Corresponding to Dose Criterion calculated in this report will be used as reference values when selecting key nuclides and for classification into concrete vault disposal when the location has not been decided. After deciding the location of the site, it is necessary to evaluate the dose based on the location conditions.
Ara, Kuniaki; Hirabayashi, Masaru*
CROSS T&T, (71), p.10 - 14, 2022/07
Development of hydrogen concentration monitors based on the application of ultrasonic technology applicable to severe accidents in nuclear reactor facilities was conducted. This paper introduces the principle and features of the application of ultrasonic technology. This paper introduces the principles and features of the ultrasonic application, and describes the performance (measurement accuracy, time response, etc.) and environmental resistance of the prototype as development results. In addition, the application of the developed technology would be introduced.
Takai, Shizuka; Namekawa, Masakazu*; Shimada, Taro; Takeda, Seiji
IEEE Transactions on Nuclear Science, 69(7), p.1789 - 1798, 2022/07
Times Cited Count：0 Percentile：0.01(Engineering, Electrical & Electronic)To reduce a large amount of contaminated concrete rubble stored in the Fukushima Daiichi Nuclear Power Station site, recycling low-radioactivity rubble within the site is a possible remedy. To promote recycling while ensuring safety, not only the average radioactivity but also the radioactivity distribution of concrete rubble should be efficiently evaluated because the details of rubble contamination caused by the accident remain unclear and likely include hotspots. However, evaluating inhomogeneous contamination of thick and/or dense materials is difficult using previous measurement systems, such as clearance monitors. This study experimentally confirmed the potential applicability of image reconstruction algorithms for radioactivity distribution evaluation in concrete rubble filled in a chamber. Radiation was measured using plastic scintillation fiber around the chamber (50 
50 40 cm
). Localized hotspots were simulated using standard sources of 
Cs, which is one of the main nuclides of contaminated rubble. The radioactivity distribution was calculated for 100 or 50 voxels (voxel size: (10 cm) or 10 10 20 cm) constituting the chamber. For 100 voxels, inner hotspots were undetected, whereas, for 50 voxels, both inner and surface hotspots were reconstructible. The distribution evaluated using the maximum likelihood expectation maximization algorithm was the most accurate; the average radioactivity was estimated within 70% accuracy in all seven cases.
Nakano, Hiroko; Fuyushima, Takumi; Tsuguchi, Akira*; Nakamura, Mutsumi*; Takeuchi, Tomoaki; Takemoto, Noriyuki; Ide, Hiroshi
JAEA-Technology 2022-007, 34 Pages, 2022/06
JAEA-Technology-2022-007.pdf:3.35MB
In order to investigate the phenomenon of stress corrosion cracking (SCC) for structural materials at the light water reactor (LWR), it is important to manage a water quality for simulating high-temperature and high-pressure water. Generally, dissolved hydrogen (DH) concentration in water loop has been controlled by the bubbling method of pure hydrogen gas or standard gas with high hydrogen concentration. However, it is necessary to equip the preventing hydrogen explosion in the area installed experimental apparatus. In general, in order to prevent accident by hydrogen, it is required to take measures such as limiting the amount of leakage, eliminating hydrogen, shutting off the power supply, and suppressing combustion before an explosion occurs. Thus, the dissolved hydrogen concentration control apparatus by electrolysis method has been developed which has two electrolysis cells to control DH concentration by electrolyzing water loop. In this study, small basic experimental devices were set up. The preliminary data were acquired regarding the simple performance of two electrolysis cells and the change of DH concentration in circulation. Based on the preliminary data, the dissolved hydrogen concentration control apparatus was designed to be connected to the high-temperature and high-pressure water loop test equipment. This report describes the test results with the small basic experimental devices for the design of the dissolved hydrogen concentration control apparatus.
Abe, Yuta; Otaka, Masahiko; Sekiya, Naoki*; Makuuchi, Etsuyo*
Hihakai Kensa, 71(2), p.69 - 74, 2022/02
no abstracts in English
Otani, Kyohei; Ueno, Fumiyoshi; Kato, Chiaki
Zairyo To Kankyo, 71(2), p.40 - 45, 2022/02
The purpose of this study is to investigate the effect of oxygen concentration in the air on the corrosion rate of carbon steel in an air/solution alternating environment in the low oxygen concentration range and to clarify the corrosion rate and corrosion mechanism of carbon steel depending on the oxygen concentration in air by the mass change of specimens before and after the corrosion test and observing the iron rust layer formed on the surface of carbon steel. The corrosion rate increases with increasing oxygen concentration in the air, and the gradient of the corrosion rate decreases gradually. The maximum erosion depth increased with increasing oxygen concentration except for the case of 1% oxygen concentration, however, the maximum erosion depth for 1% oxygen concentration was larger than that for 5% air oxygen concentration.
Sasa, Toshinobu
Kasokuki, 18(4), p.233 - 240, 2022/01
Lead bismuth eutectic alloy (LBE) is a promising option as a spallation target for accelerator-driven transmutation systems (ADS) to reduce the radiological toxicity from long-lived radioactive waste. LBE is a heavy metal and has suitable characteristics both as a spallation target and as a coolant for transmutation systems. However, LBE is also known as a highly corrosive with structural materials. In this paper, technological developments to overcome the issue, the latest research activities such as hightemperature operation and oxygen concentration control to ensure corrosion resistance, are introduced together with the outline of the target for ADS.
Moriguchi, Yuichi*; Sato, Yosuke*; Morino, Yu*; Goto, Daisuke*; Sekiyama, Tsuyoshi*; Terada, Hiroaki; Takigawa, Masayuki*; Tsuruta, Haruo*; Yamazawa, Hiromi*
KEK Proceedings 2021-2, p.21 - 27, 2021/12
no abstracts in English
Otani, Kyohei; Kato, Chiaki
Zairyo To Kankyo, 70(12), p.480 - 486, 2021/12
This is a comprehensive paper of the corrosion of carbon steel in air/solution alternating condition. From cross-sectional observation and analysis of the iron rust layer formed on the surface of carbon steel in the alternating condition, it was found that a multilayered iron rust layer composed of red rust layer (-FeOOH), rust crust layer (Fe
O
), inner crystal (FeO), and inner rust layer was formed on carbon steel. The multi-layered iron rust layer would accelerate the cathodic oxygen reduction reaction, and the reason why the corrosion rate of the carbon steel in the alternating condition was accelerated. The effect of artificial seawater (ASW) composition on the corrosion rate of carbon steel in air/solution alternating condition was investigated. It was found that the corrosion rate increased with increasing concentration from pure water to 200 times diluted ASW, and decreased with increasing concentration from 20 times diluted ASW to no diluted ASW. The Mg and Ca ions in ASW precipitated on the reaction interface and formed a metal cation layer, which inhibited the oxygen reduction reaction, and thus the corrosion of carbon steel was inhibited in the highly concentrated ASW.
Asakura, Kazuki; Shimomura, Yusuke; Donomae, Yasushi; Abe, Kazuyuki; Kitamura, Ryoichi; Miyakoshi, Hiroyuki; Takamatsu, Misao; Sakamoto, Naoki; Isozaki, Ryosuke; Onishi, Takashi; et al.
JAEA-Review 2021-020, 42 Pages, 2021/10
JAEA-Review-2021-020.pdf:2.95MB
The disposal of radioactive waste from the research facility need to calculate from the radioactivity concentration that based on variously nuclear fuels and materials. In Japan Atomic Energy Agency Oarai Research and Development Institute, the study on considering disposal is being advanced among the facilities which generate radioactive waste as well as the facilities which process radioactive waste. This report summarizes a study result in FY2020 about the evaluation method to determine the radioactivity concentration in radioactive waste on Oarai Research and Development Institute.
Sun, Haomin; Shibamoto, Yasuteru; Hirose, Yoshiyasu; Kukita, Yutaka
Journal of Nuclear Science and Technology, 58(9), p.1048 - 1057, 2021/09
Times Cited Count：4 Percentile：56.94(Nuclear Science & Technology)no abstracts in English
Sugaya, Toshikatsu; Abe, Daichi*; Okada, Shota; Nakata, Hisakazu; Sakai, Akihiro
JAEA-Technology 2021-004, 79 Pages, 2021/05
JAEA-Technology-2021-004.pdf:2.86MBJAEA-Technology-2021-004(errata).pdf:0.38MB
JAEA has aims to carry out near surface disposal of low-level radioactive waste generated from research, medical, and industrial facilities. Therefore, radioactivity concentration corresponding to dose criteria of near surface disposal for 220 nuclides in the waste were calculated for the purpose of discussion for radioactivity limits between trench and concrete vault disposal, and key nuclides related to them. We calculated the radioactivity concentrations with consideration of not only the exposure pathways used at calculation of the radioactivity concentration limits of waste packages for near surface disposal by Nuclear Safety Commission but also ones used at the concentration limits for intermediate depth disposal. We also assumed the capacities of the disposal facilities as 44,000 m for pit disposal and 150,000 m for trench disposal. The radioactivity concentrations calculated in this report is used as the reference values because the disposal site has not been decided yet. Addition to this, the radioactivity concentrations will be revised according to circumstances of development of disposal facilities and so on. In the future, we will decide the radioactivity and radioactive concentration of a waste package described in the license application documents based on the dose assessment taken into consideration the disposal site conditions.
Saito, Shigeru; Wan, T.*; Okubo, Nariaki; Obayashi, Hironari; Watanabe, Nao; Ohdaira, Naoya*; Kinoshita, Hidetaka; Yamaki, Kenichi*; Kita, Satoshi*; Yoshimoto, Hidemitsu*; et al.
JPS Conference Proceedings (Internet), 33, p.011041_1 - 011041_6, 2021/03
An Accelerator Driven System (ADS) for waste transmutation investigated in JAEA employs lead-bismuth eutectic (LBE) as a neutron production target material and coolant. The neutrons are to be produced via the spallation with 1.5 GeV proton beam injection. As materials irradiation data are important for ADS development, JAEA plans to construct an irradiation facility with LBE neutron production target in J-PARC. There are many technical issues on LBE for practical use. In JAEA, various R&Ds are being carried out. Concerning corrosion study, conditioning operation and functional tests of OLLOCHI started. Oxygen concentration control technology has also developing. In the large scale LBE loop experiment, the operation for steady state and transient experiments was performed by using IMMORTAL. In the area of instrument, development of ultrasonic flow meter and freeze seal valve are progressing as a key technology for the LBE loop system. Investigation of behavior of impurities in LBE, which is important for design of the irradiation facility, started. In this paper, the status of the LBE studies and experimental plan will be presented.
Sasa, Toshinobu; Saito, Shigeru; Obayashi, Hironari; Ariyoshi, Gen
JPS Conference Proceedings (Internet), 33, p.011051_1 - 011051_6, 2021/03
To realize Accelerator-driven system (ADS) for minor actinide transmutation, JAEA proposes to construct the Proton Irradiation Facility in J-PARC. The facility is planned to solve technical issues for safe application of Lead-bismuth Eutectic Alloy (LBE). The 250 kW LBE spallation target will be located in the facility to prepare material irradiation database by both proton and neutron irradiation in the temperature range for typical LBE-cooled ADS. Various studies for important technologies required to build the facilities are investigated such as oxygen concentration control, instruments development, remote handling techniques for target maintenance, and spallation target design. The large scale LBE loops for mock up the 250 kW LBE spallation target and material corrosion studies are also manufactured and applied to various experiments. The latest status of 250 kW LBE spallation target design works will be summarized.
Sun, Haomin; Porcheron, E.*; Magne, S.*; Leroy, M.*; Dhote, J.*; Ruffien Ciszak, A.*; Bentaib, A.*
Proceedings of OECD/NEA Specialist Workshop on Advanced Measurement Method and Instrumentation for enhancing Severe Accident Management in an NPP addressing Emergency, Stabilization and Long-term Recovery Phases (SAMMI 2020) (Internet), 10 Pages, 2020/12
Bentaib, A.*; Janin, T.*; Porcheron, E.*; Magne, S.*; Leroy, M.*; Dhote, J.*; Ruffien Ciszak, A.*; Sun, Haomin
Proceedings of OECD/NEA Specialist Workshop on Advanced Measurement Method and Instrumentation for enhancing Severe Accident Management in an NPP addressing Emergency, Stabilization and Long-term Recovery Phases (SAMMI 2020) (Internet), 6 Pages, 2020/12
